"Stability" is not a bright line. The "1.0 caliber" rule is just a rule of thumb. I don't even think it's a good one. I've written elsewhere about how I think the proper denominator should logically involve the length of the rocket rather than the diameter. I've seen references to "real" scientific literature that supports that hypothesis, I just haven't read far enough to find that basis myself. On a forum I used to read, one person's sig was something like, "Never use a rule of thumb. It's prone to mildew and invariably not straight."
One of the problems with design of experiment for stability of an aerodynamically stabilized rocket is that it is about the response to disturbances and how the rocket recovers. The nature and magnitude of disturbance may differ enough from flight to flight (some variance systematic, predictable, measurable and some completely random) to generate a large scatter in the results. Ideally, you want a solution that's not marginal, but robust. On the other hand, an overstable rocket also leads to a variety of problems. So there's a "zone" of optimized compromise. The sweet spot of that zone may vary depending on conditions, and it will vary depending on motor characteristics. The "optimum" answer across the range of conditions one might fly in may involve changeable ballast.
All that is to say, I suspect a large amount of work could be done and money spent to generate data that is only directionally useful for a particular rocket configuration, and we kinda already have that level and type of information available.